Synthesis, characterization and energy gap of silica quantum dots from rice husk

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Ely Setyo Astuti, Achmad As'ad Sonief, M. Sarosa, Ngafwan Ngafwan, I.N.G. Wardana

2022 Bioresource Technology Reports Vol. 20 Article Cited by 14 Quartile

Abstract

This study aimed to reveal roles of KOH and HCl in a synthesis process of Silica Quantum Dots (Si-QDs) from environmentally friendly rice husk waste, the morphological characteristics, size and crystal structure of particles as well as the energy gap of Si-QDs. The results showed that High Energy Milling (HEM) caused electron excitation, delocalized bonding, nanocrack and fracture. KOH played a role in producing Si-QDs sizes around 0.386–2.5 nm. The most efficient hexagonal crystal structure absorbed the peak wavelength of about 250–400 nm and glowed a purplish-blue color. The Si-QDs produced Si and O content was 97 % with 3 % of K, Fe, and Ca impurities. The obtained energy gap 1.59–2.36 eV and HOMO-LUMO 127 99.5 kcal/mol. The smaller size of Si QDs, the higher energy gap which was associated with the quantum confinement effect. © 2022 Elsevier Ltd

Affiliations

Doctoral Student, Department of Mechanical Engineering, Brawijaya University, Jl. MT. Haryono no 167, East Java, Malang, 65145, Indonesia; Department of Mechanical Engineering, Brawijaya University, Jl. MT. Haryono 167, East Java, Malang, 65145, Indonesia; State Polytechnic of Malang, Jl. Soekarno Hatta 9, East Java, Malang, 65141, Indonesia; Department of Mechanical Engineering, Muhammadiyah University of Surakarta, Jl. A. Yani, Mendungan, Pabelan, Kartasura, Central Java, Sukoharjo, 67169, Indonesia